Abstract
The isotope shifts and hyperfine splitting have been measured in 144-154Sm I using the crossed-beam laser fluorescence method. Transitions at 598.98 nm and 570.68 nm were investigated for all isotopes except 146Sm and 153Sm, in which measurements were only obtained at 570.68 nm. Laser-induced fluorescence has not previously been reported for 145Sm: the hyperfine structure for the ground state of this isotope leads to mu =1.123 mu N, Q(spectroscopic)=-0.60e2b2 and delta (r2) (144-145)=0.11 fm2. The magnetic dipole and electric quadrupole moments of the odd isotopes and the changes in mean square radii of the even ones are shown to be consistent with the information obtained from nuclear spectroscopy.