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The role of quantal fluctuations in the optical response of small metal clusters
Journal article   Peer reviewed

The role of quantal fluctuations in the optical response of small metal clusters

A Fortini, M Mazzola, A Mina, D Provasi, G Coló, G Onida, HE Roman and RA Broglia
Journal of Physics B: Atomic, Molecular and Optical Physics, Vol.38(11), pp.1581-1589
14/06/2005

Abstract

We present an ab initio calculation of the line shape of the photoabsorption spectrum of Na8 and Na+9 clusters at zero temperature, including the polarization effect driven by the electron-plasmon coupling, together with the electron-phonon coupling. The electron-plasmon coupling is found to yield a significant lowering of the energy centroid of the plasmons, whereas the main effect the electron-phonon coupling has is to smooth the spectrum. © 2005 IOP Publishing Ltd.

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