Abstract
The highly selective, intermediate-energy heavy-ion-induced neutron-pickup reaction, in combination with γ-ray spectroscopy using the γ-ray energy-tracking in-beam nuclear array (GRETINA), is shown to provide reliable relative spectroscopic strengths for high-ℓ orbitals in nuclei more neutron rich than the projectile. The reaction mechanism gives a significant final-state-spin alignment that is validated through γ-ray angular-distribution measurements enabled by the position sensitivity of GRETINA. This is the first time that γ-ray angular distributions could be extracted from a high-luminosity, fast-beam reaction other than inelastic scattering. This holds great promise for the restriction and assignment of Jπ quantum numbers in exotic nuclei. We advance this approach to study the crucial N=28 shell closure and extract the ratio g9/2:f5/2 of bound neutron single-particle strengths in Ca49, a benchmark for emerging multi-shell ab initio and configuration-interaction theories that are applicable along the Ca isotopic chain.